Gold-catalyzed post-Ugi alkyne hydroarylation for the synthesis of 2-quinolones

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Date

2018-10-04

Authors

Du, Xiaochen
Huang, Jianjun
Nechaev, Anton A.
Yao, Ruwei
Gong, Jing
Van der Eycken, Erik V.
Pereshivko, Olga P.
Peshkov, Vsevolod A.

Journal Title

Journal ISSN

Volume Title

Publisher

Beilstein J. Org. Chem.

Abstract

A series of propargylamides containing an electron-rich benzene ring was prepared through the Ugi reaction of 3,5-dimethoxyaniline with various propiolic acids, aldehydes and isocyanides. Subjecting these adducts to a gold-catalyzed intramolecular alkyne hydroarylation process allowed to efficiently construct the 2-quinolone core bearing a branched substituent on the nitrogen atom...

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Keywords

gold catalysis, hydroarylation, Ugi reaction

Citation

Du, X.; Huang, J.; Nechaev, A. A.; Yao, R.; Gong, J.; Van der Eycken, E. V.; Pereshivko, O. P.; Peshkov, V. A. Beilstein J. Org. Chem. 2018, 14, 2572–2579. doi:10.3762/bjoc.14.234

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